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Seismic tomographic models based only on wave velocities have limited ability to distinguish between a thermal or compositional origin for Earth’s 3D structure1 . Complementing wave velocities with attenuation observations can make that distinction, which is fundamental for understanding mantle convection evolution. However, global 3D attenuation models are only available for the upper mantle at present2–5. Here we present a 3D global model of attenuation for the whole mantle made using whole-Earth oscillations, constraining even spherical harmonics up to degree four. In the upper mantle, we find that high attenuation correlates with low velocity, indicating a thermal origin, in agreement with previous studies6,7. In the lower mantle, we find the opposite and observe the highest attenuation in the ‘ring around the Pacific’, which is seismically fast, and the lowest attenuation in the large low-seismic-velocity provinces (LLSVPs). Comparing our model with wave speeds and attenuation predicted by a laboratory-based viscoelastic model8 suggests that the circum-Pacific is a colder and small-grain-size region9, surrounding the warmer and large-grain-size LLSVPs. Viscosities calculated for the inferred variations in grain size and temperature confirm LLSVPs as long-lived, stable features10